Time-dependent nucleation during reheating of a rapidly quenched glass

V. A. Shneidman

doi:10.1063/1.468706

Time-dependent nucleation during reheating of a rapidly quenched glass

V. A. Shneidman

Research output: Contribution to journal › Article › peer-review

14 Scopus citations

Abstract

If the temperature of a glass is continuously increased nucleation can start only after the nascent nuclei are able to escape the advancing critical size. In case the starting temperature T† exceeds the temperature of the maximum nucleation rate, corrections to the steady-state values of the number of nucleated particles become dramatic. Analytical estimations are confirmed with high accuracy by numerical solutions of the time-dependent Becker-Döring equation.

Original language	English (US)
Pages (from-to)	1791-1795
Number of pages	5
Journal	The Journal of Chemical Physics
Volume	102
Issue number	4
DOIs	https://doi.org/10.1063/1.468706
State	Published - 1995
Externally published	Yes

All Science Journal Classification (ASJC) codes

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1063/1.468706

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title = "Time-dependent nucleation during reheating of a rapidly quenched glass",

abstract = "If the temperature of a glass is continuously increased nucleation can start only after the nascent nuclei are able to escape the advancing critical size. In case the starting temperature T† exceeds the temperature of the maximum nucleation rate, corrections to the steady-state values of the number of nucleated particles become dramatic. Analytical estimations are confirmed with high accuracy by numerical solutions of the time-dependent Becker-D{\"o}ring equation.",

author = "Shneidman, {V. A.}",

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AU - Shneidman, V. A.

PY - 1995

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N2 - If the temperature of a glass is continuously increased nucleation can start only after the nascent nuclei are able to escape the advancing critical size. In case the starting temperature T† exceeds the temperature of the maximum nucleation rate, corrections to the steady-state values of the number of nucleated particles become dramatic. Analytical estimations are confirmed with high accuracy by numerical solutions of the time-dependent Becker-Döring equation.

AB - If the temperature of a glass is continuously increased nucleation can start only after the nascent nuclei are able to escape the advancing critical size. In case the starting temperature T† exceeds the temperature of the maximum nucleation rate, corrections to the steady-state values of the number of nucleated particles become dramatic. Analytical estimations are confirmed with high accuracy by numerical solutions of the time-dependent Becker-Döring equation.

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U2 - 10.1063/1.468706

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JO - The Journal of Chemical Physics

JF - The Journal of Chemical Physics

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ER -

Time-dependent nucleation during reheating of a rapidly quenched glass

Abstract

All Science Journal Classification (ASJC) codes

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