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Topological magneto-optical Kerr effect without spin-orbit coupling in spin-compensated antiferromagnet

  • Camron Farhang
  • , Weihang Lu
  • , Kai Du
  • , Yunpeng Gao
  • , Junjie Yang
  • , Sang Wook Cheong
  • , Jing Xia

Research output: Contribution to journalArticlepeer-review

Abstract

The magneto-optical Kerr effect (MOKE), the differential reflection of oppositely circularly polarized light, has traditionally been associated with relativistic spin-orbit coupling (SOC), which links a particle’s spin with its orbital motion. In ferromagnets, large MOKE signals arise from the combination of magnetization and SOC, while in certain coplanar antiferromagnets, SOC-induced Berry curvature enables MOKE despite zero net magnetization. Theoretically, large MOKE can also arise in a broader class of magnetic materials with compensated spins, without relying on SOC - for example, in systems exhibiting real-space scalar spin chirality. The experimental verification has remained elusive. Here, we demonstrate such a SOC- and magnetization-free MOKE in the noncoplanar antiferromagnet Co1/3TaS2. Using a Sagnac interferometer microscope, we image domains of scalar spin chirality and their reversal. Our findings establish experimentally a new mechanism for generating large MOKE signals and position chiral spin textures in compensated magnets as a compelling platform for ultrafast, stray-field-immune opto-spintronic applications.

Original languageEnglish (US)
Article number3386
JournalNature communications
Volume17
Issue number1
DOIs
StatePublished - Dec 2026

All Science Journal Classification (ASJC) codes

  • General Chemistry
  • General Biochemistry, Genetics and Molecular Biology
  • General
  • General Physics and Astronomy

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